Well, after searching a bit, I found this,
http://www.linuxhomenetworking.com/wiki/index.php/Quick_HOWTO_:_Ch28_:_Managing_Disk_Usage_with_Quotas#Edit_The_User.27s_Quota_Information. Which led me to this:
sudo edquota -u <my username>
So now I can connect to shares without the 100mb limit issue. Here's the real issue: I have user quotas disabled through the Zentyal Dashboard (I'm assuming Users and Groups-> User Template -> Default user quota: Disabled), so something is not being flipped, even after I've tried changing it on/off.
Also, to note, this is not a user share, so why would my user have a quota? I would expect users to have quotas on their home shares, but not a regular share? Is the user quota supposed to be a gobal thing across all shares? To me that doesn't really make sense from an admin standpoint.
Also, for kicks, I took a look to see if the share had Group Quotas set:
root@samba:/var/log# sudo edquota -g /home/samba/shares/<share>/
edquota: group /home/samba/shares/techops/ does not exist.
So, the next thing was to look at /etc/fstab according to the link:
# <file system> <mount point> <type> <options> <dump> <pass>
proc /proc proc nodev,noexec,nosuid 0 0
/dev/mapper/samba-root / ext4 errors=remount-ro,usrquota,grpquota,acl 0 1
Bingo, I see the userquota is enabled there. So, I am debating here, but if I want to just disable quotas for everyone in one shot, should I just pull the userquota from the above? Any guidance would be very much appreciated.